Great songs for a duet/two-part harmony?

It's very possible to learn to sing well. You just need to know the right methods. Learn here https://tinyurl.im/aH6mx Singing teachers will cost money and can be expensive so they're not for everyone. Singing can be learned so it's not an "either you have it or you don't" kind of thing. Whether you sound like crap or you're decent, I recommend this singing course. It's one of the best methods to learn to sing well in a short amount of time. It's all about using efficient techniques that work.

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Nowadays you can learn how to sing over the internet. You can check out the best singing video lessons here: https://www.goobypls.com/r/rd.asp?gid=541

The videos are very easy to follow and to my surprise extremely helpful even for advanced singers. For beginners I would have to say this is a gold mine. I was able to improve my singing, voice tone and range in just under two weeks and I am an advanced musician...

I wanted to go to a singing teacher but that would have cost me over 1500 bucks .... every month!

Following a course online is much cheaper!

If you want to know a very good vocal coach try to visit https://tr.im/KkFOP an online vocal coaching tutorial. Everything, ranging from breathing fundamentals, vocalizing exercises, techniques on singing high and low notes, how to not go off-key/out of tune/off-sync, musicianship and music theory, proper diction and articulation, and a lot more are covered, all in our native language. It can be quite technical in nature, but it really helps since it covers the musical aspect of singing deeply and not just concentrates on how to impress people with your vocal range, riffs and runs and other cliches that do not necessarily make one a complete vocalist.

You should try checking out...

Of Monsters and Men

VersaEmerge

Alex and Sierra (they're on the X Factor USA and you can see how they arranged the covers of their songs)

Boyce Avenue

You can also pretty much pick any song you like and harmonize :)

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I think you chose a really good one there with Simon & Garfunkel. They were fantastic. You might also want to look into songs by Chad & Jeremy ("A Summer Song"), and Seals & Crofts ("Summer Breeze" & "Diamond Girl") .... beautiful tunes ... great harmonies.

There's this Snow Patrol song that's not too high that they did with Martha Wainwright. It's called Set the Fire to the Third Bar.

Gang of Rhythm by Walk off the Earth

"Close My Eyes Forever" by Ozzy Osbourne and Lita Ford. Great duo. Check it out on you tube.